This special issue includes papers based on recent field campaigns, including US Department of Energy Aerosol and Cloud Experiments in Eastern North Atlantic (ACE-ENA), NASA North Atlantic Aerosols and Marine Ecosystems Study (NAAMES), and the North Atlantic Climate System Integrated Study (ACSIS), and long-term measurements from observatories (e.g., the Atmospheric Radiation Measurement Eastern North Atlantic site on Graciosa Island in the Azores). Presently the responses of marine low-cloud systems to changes in atmospheric greenhouse gases and aerosols are major sources of uncertainty that limit our ability to predict future climate. Major contributions to this uncertainty derive from poor understanding of the cloud responses to aerosol changes and the natural aerosol state that is being perturbed by anthropogenic emissions. One overarching scientific objective of these recent field campaigns is to understand key processes that drive the properties and interactions of aerosol and clouds under representative meteorological and cloud conditions. Another important focus is to validate and improve ground-based retrieval algorithms using comprehensive in situ aircraft measurements. This will lead to high-quality, long-term datasets from the routine ground-based remote sensing, which allow greater statistical reliability in the observed properties and relationships among aerosols, clouds, and precipitation than is possible with the aircraft measurements alone.

With a wide variety of aerosol optical, physical, and chemical properties, China offers a test bed for the study of aerosol processes and techniques leading to a better understanding of aerosol properties. Aerosol concentrations in the southeast of China are periodically among the highest in the world, while at other times they are relatively low. The prevailing aerosol chemical composition (e.g., sulfate, nitrate, black carbon, brown carbon, particulate organic matter, sea salt) also changes significantly with the quick evolution of both the economy and society, along with the government’s strong environmental actions. The complex mechanisms of the secondary formation of aerosols and haze-fog interaction are still not well understood in this important region. In areas other than the southeast of China, topography determines the aerosol concentrations, which are consistently high. Examples are Sichuan Province or the Guanzhong Basin, i.e. large basins surrounded by high mountains. Furthermore, the large deserts in the west and north of China are strong sources of dust particles influencing the aerosol properties over a large part of the country. There are however also large areas with relatively low aerosol loading, in particular in mountainous areas and over the high plateaus such as Tibet. Aerosol chemical properties in the center and east of China still need to be clarified both geographically and temporally, e.g. distinguish spectrally absorbing components like mineral dust and brown carbon from remote sensing observations. Anthropogenic emissions of aerosols and precursor gases have a large influence on aerosol, in regards to both chemical and physical properties, and consequently optical properties, and their effects can be augmented by the transport of aerosol from elsewhere, such as carbonaceous particles from biomass burning aerosol and dust particles emitted from the deserts. The complex mechanisms and intrinsic relations of aerosol chemistry and physics, and their impacts on optical properties, need better interpretation based on comprehensive observation and analysis. Weather conditions have a large influence on the formation of haze, and haze episodes occur more and more frequently. The influence of large-scale weather systems such as the monsoon or the Siberian high may result in inter-annual variations in different regions of China. In particular the progress of the monsoon from south to north during spring and summer, and back in the autumn, results in strong variations in aerosol content.

In this special issue we focus on the application of remote sensing techniques using both ground-based and satellite measurements to study the temporal and spatial variations in aerosol properties over China on different scales. Results from campaigns in the Taklamakan Desert (Kashi), on the Tibetan Plateau, and other remote areas such as the NE of China are contrasted with those from densely populated and industrialized urban areas in the east of China. The special issue aims to bring together results from different projects such as Kashi, MOST, and regional air quality studies. Contributions are solicited on aerosol optical, physical, and chemical properties inferred from remote sensing observations and related optical techniques, and the spatial and temporal variations in these properties across China, with emphasis on processes leading to the observed differences, including the influence of meteorological conditions and large-scale weather systems.

The Wave-driven ISentropic Exchange (WISE) mission is a collaborative research project to investigate transport and mixing processes in the upper troposphere and the lower stratosphere (UTLS) over the Atlantic. Headed by Forschungszentrum Jülich GmbH and the Johannes Gutenberg University of Mainz, 14 measurement flights were conducted with the high-altitude research aircraft HALO in September and October 2017 from Shannon, Ireland. Further partners providing instrumentation were the Karlsruhe Institute for Technology (KIT), the German Aerospace Center (DLR), the universities of Heidelberg, Frankfurt am Main, and Wuppertal, and the German National Metrology Institute. The scientific flights were supported by a team of about 90 persons.

The main objective of this project is to study the relation between chemical composition and the dynamical structure of the UTLS with a focus on the following topics: (i) interrelation of the tropopause inversion layer (TIL) and trace gas distribution, (ii) role of planetary wave breaking for water vapor transport into the extratropical lower stratosphere, (iii) role of halogenated substances for ozone and radiative forcing in the UTLS region, and (iv) occurrence and effects of sub-visual cirrus (SVC) in the lowermost stratosphere.

The special issue mainly includes papers from the airborne measurement campaign itself but is also open to other studies close to the topic. This includes both advanced scientific analyses of observational and measured data during the campaign as well as related climatological studies, but also manuscripts based on instrumental developments.

The ISTP11 AMT special issue aims at collecting original papers from the 11th Edition of the International Symposium on Tropospheric Profiling (ISTP11) as well as additional contributions fitting well within the scope of tropospheric profiling. The main topics will cover new algorithms, instrumental techniques and synergy to retrieve atmospheric profiling of state parameters and consituents (clouds, aerosols and trace gazes), improved understanding of tropospheric processes thanks to innovative dataset of tropospheric profiles and the use of experimental data to improve numerical weather prediction (model evaluation, advances in modelling and data assimilation).

In order to improve our current knowledge on the budgets of the two most important anthropogenic greenhouse gases, CO₂ and CH₄, a co-ordinated measurement campaign in the central European region was successfully carried out in May-June 2018 with the German research aircraft HALO and two smaller Cessna aircraft as its main experimental platforms. The goal of CoMet is to combine a suite of state-of-the-art airborne active (lidar) and passive remote sensors (spectrometer) with in situ instruments to provide regional-scale data about greenhouse gases (GHGs) which are urgently required for their accurate modelling.

During the intensive observation period, HALO research flights were performed along extended latitudinal transects to capture GHG gradients, over known regions of strong emissions, and over the ground-based remote-sensing sites of the Total Carbon Column Observing Network (TCCON). While HALO provides a larger-scale picture, the two Cessna aircraft concentrated on a region of prime interest: the Upper Silesian Coal Basin in Poland, which, due to hard coal mining activities, is one of the hot spots of anthropogenic methane emissions in Europe. Here, a variety of ground-based instruments additionally supported the CoMet mission: FTIR spectrometers, wind lidars, mobile vans, and small drones provided valuable information to quantify CH₄ emissions from coal mining activities. A model infrastructure (regional inverse modelling, chemistry-climate modelling with regional refinement) has been employed in forecast mode to optimize flight strategies and is now used to hindcast the campaign period to evaluate GHG fluxes and transport. The CoMet mission is also part of validation activities for existing passive remote sounding GHG satellites (GOSAT, Sentinel-5P, and OCO-2) and preparation of the first active CH₄ satellite mission MERLIN. For that reason, the CHARM-F lidar developed at DLR as an airborne MERLIN demonstrator was one of the key instruments. In addition, CoMet is intended to investigate methodologies for the synergistic combination for GHG measurements using lidar and passive remote sensing.